Optical measurements of spin noise as a high resolution spectroscopic tool (1206.4168v1)

Abstract: The intrinsic fluctuations of electron spins in semiconductors and atomic vapors generate a small, randomly-varying "spin noise" that can be detected by sensitive optical methods such as Faraday rotation. Recent studies have demonstrated that the frequency, linewidth, and lineshape of this spin noise directly reveals dynamical spin properties such as dephasing times, relaxation mechanisms and g-factors without perturbing the spins away from equilibrium. Here we demonstrate that spin noise measurements using wavelength-tunable probe light forms the basis of a powerful and novel spectroscopic tool to provide unique information that is fundamentally inaccessible via conventional linear optics. In particular, the wavelength dependence of the detected spin noise power can reveal homogeneous linewidths buried within inhomogeneously-broadened optical spectra, and can resolve overlapping optical transitions belonging to different spin systems. These new possibilities are explored both theoretically and via experiments on spin systems in opposite limits of inhomogeneous broadening (alkali atom vapors and semiconductor quantum dots).