Penning-Trap Mass Measurement of Helium-4

Abstract: Light-Ion Trap (LIONTRAP), a high-precision Penning-trap mass spectrometer, was used to determine the atomic mass of $^{4}$He. Here, we report a 12 parts-per-trillion measurement of the mass of a $^{4}$He$^{2+}$ ion, $m(^{4}\text{He}^{2+}$) = $4.001:506:179:651 (48)$ u. From this, the atomic mass of the neutral atom can be determined without loss of precision: $m(^{4}\text{He})$ = $4.002:603:254:653 (48)$ u. This result is slightly more precise than the current CODATA18 literature value but deviates by 6.6 standard deviations. This is a post-peer-review, pre-copy edit version of an article published in PRL. The final version is available online at https://doi.org/10.1103/PhysRevLett.131.093201.