Deforming Active Droplets in Viscoelastic Media

Abstract: To mimic the motion of biological swimmers in bodily fluids, a novel experimental system of micellar solubilization driven active droplets in a visco-elastic polymeric solution is presented. The visco-elastic nature of the medium, characterized by the Deborah number (De), is tuned by varying the surfactant (fuel) and polymer concentration in the ambient medium. At moderate De, the droplet exhibits a steady deformed shape, markedly different from the spherical shape observed in Newtonian media. A theoretical analysis based on the normal stress balance at the interface is shown to accurately predict the droplet shape. With a further increase in De, time-periodic deformations accompanied by oscillatory transitions in swimming modes are observed. The study unveils the rich complexity in the motion of active droplets in viscoelastic fluids, which has been hitherto unexplored.