Efficient conversion of closed-channel dominated Feshbach molecules of $^{23}$Na$^{40}$K to their absolute ground state (2106.10089v2)

Abstract: We demonstrate the transfer of $^{23}$Na$^{40}$K molecules from a closed-channel dominated Feshbach-molecule state to the absolute ground state. The Feshbach molecules are initially created from a gas of sodium and potassium atoms via adiabatic ramping over a Feshbach resonance at 78.3$\,$G. The molecules are then transferred to the absolute ground state using stimulated Raman adiabatic passage with an intermediate state in the spin-orbit-coupled complex $|c^3 \Sigma^+, v=35, J=1 \rangle \sim |B^1\Pi, v=12, J=1\rangle$. Our measurements show that the pump transition dipole moment linearly increases with the closed-channel fraction. Thus, the pump-beam intensity can be two orders of magnitude lower than is necessary with open-channel dominated Feshbach molecules. We also demonstrate that the phase noise of the Raman lasers can be reduced by filter cavities, significantly improving the transfer efficiency.