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Fractional viscoelastic models for power-law materials (2003.07834v3)

Published 17 Mar 2020 in cond-mat.soft, physics.bio-ph, q-bio.QM, and q-bio.TO

Abstract: Soft materials often exhibit a distinctive power-law viscoelastic response arising from broad distribution of time-scales present in their complex internal structure. A promising tool to accurately describe the rheological behaviour of soft materials is fractional calculus. However, its use in the scientific community remains limited due to the unusual notation and non-trivial properties of fractional operators. This review aims to provide a clear and accessible description of fractional viscoelastic models for a broad audience, and to demonstrate the ability of these models to deliver a unified approach for the characterisation of power-law materials. The use of a consistent framework for the analysis of rheological data would help classify the empirical behaviours of soft and biological materials, and better understand their response.

Citations (203)

Summary

Insights into Fractional Viscoelastic Models for Power-Law Materials

The paper "Fractional viscoelastic models for power-law materials" offers an in-depth exploration of the use of fractional calculus in modeling the rheological properties of materials exhibiting power-law viscoelastic behaviors. These materials, characterized by their broad distribution of time-scales, present a unique challenge to traditional viscoelastic models that rely on differential equations with integer-order derivatives. The paper advocates for a shift towards fractional viscoelastic models, highlighting their ability to provide a consistent framework for characterizing complex materials while maintaining a manageable number of parameters.

The research is extensive and centers on fractional calculus, a mathematical domain that extends the notion of differentiation to non-integer orders—an approach that naturally aligns with the observed power-law behaviors in soft and biological materials. Fractional derivatives, specifically Caputo derivatives, are employed to model material responses, leading to the introduction of a conceptual element termed the "springpot." This element is able to describe a continuum of material behaviors ranging from purely elastic to viscous, depending on the fractional order of differentiation.

The rationale for adopting fractional viscoelastic models stems from the limitations of traditional spring-dashpot models, which typically require a multitude of parameters to approximate power-law behaviors accurately. While these traditional models can make empirical fittings through multiple discrete time scales, they often lack the capacity for clear physical interpretation and extrapolation beyond the observed data ranges. In contrast, fractional models, by design, offer a more integrated and concise approach, accommodating the continuous distribution of relaxation and creep time scales seen in power-law materials.

Notably, the paper makes several significant claims through empirical demonstrations. Firstly, it identifies that many empirical functions used in previous literature can be equated or mapped onto fractional equivalents, thus simplifying and unifying past approaches under a fractional framework. This is exemplified by the reinterpretation of the structural damping model and other ad-hoc power-law representations, which correspond directly to special cases of fractional models like the fractional Kelvin-Voigt or Maxwell models.

The paper further explores practical applications, showing with rigorous data analysis how fractional models can more effectively capture the viscoelastic characteristics of diverse materials, from biological tissues and cells to synthetic polymers. A cornerstone of the paper is the demonstration of how fractional models significantly alleviate the need for excessive parameters without sacrificing predictive accuracy—a critical advancement for experimental contexts and theoretical predictions in the materials science community.

In terms of implications, the adoption of fractional viscoelastic models holds considerable promise for enhancing the consistency and comparability of rheological studies. By promoting a unified approach for modeling power-law materials, this research not only provides practical tools for scientists and engineers but also encourages a theoretical shift towards recognizing fractional calculus as a standard component of viscoelastic modeling.

Looking towards the future, this paper sets the stage for further integration of fractional models in complex, nonlinear regimes, potentially crossing into the field of non-linear fractional viscoelasticity. Additionally, expanding computational tools for simulating fractional models could further encourage their adoption and broaden their applicability across various disciplines, from tissue engineering and biomechanics to geosciences and material fabrication. By doing so, the research pivots the discourse from purely empirical modeling to a more theory-driven understanding of power-law materials—a vital step for advancing both the science of complex materials and its practical applications.

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