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Probing the Ultimate Plasmon Confinement Limits with a Van der Waals heterostructure (1804.01061v1)

Published 3 Apr 2018 in cond-mat.mes-hall and quant-ph

Abstract: The ability to confine light into tiny spatial dimensions is important for applications such as microscopy, sensing and nanoscale lasers. While plasmons offer an appealing avenue to confine light, Landau damping in metals imposes a trade-off between optical field confinement and losses. We show that a graphene-insulator-metal heterostructure can overcome that trade-off, and demonstrate plasmon confinement down to the ultimate limit of the lengthscale of one atom. This is achieved by far-field excitation of plasmon modes squeezed into an atomically thin hexagonal boron nitride dielectric h-BN spacer between graphene and metal rods. A theoretical model which takes into account the non-local optical response of both graphene and metal is used to describe the results. These ultra-confined plasmonic modes, addressed with far-field light excitation, enables a route to new regimes of ultra-strong light-matter interactions.

Citations (291)

Summary

  • The paper demonstrates plasmon confinement down to a single atom's scale using graphene-hBN heterostructures coupled with metal rods.
  • Advanced FDTD and semi-analytical simulations validate both local and non-local optical responses, confirming the experimental framework.
  • This breakthrough paves the way for enhanced light-matter interactions, improved molecular sensing, and more efficient photodetectors.

Probing the Ultimate Plasmon Confinement Limits with a Van der Waals Heterostructure

The paper explores the plasmon confinement limits using a van der Waals heterostructure, showing potential advancements in nano-optic applications. Through the integrative use of graphene-insulator-metal (GIM) heterostructures, the paper advances previous boundaries of light confinement at atomic scales, thereby paving the way for novel optoelectronic properties. This is achieved by encapsulating graphene in an atomically thin dielectric and using metal rods to achieve significant plasmonic confinements.

Key findings in the paper highlight the realization of plasmon confinement down to a single atom's scale, achieved by employing a heterostructure comprising graphene and spacers of hexagonal boron nitride (h-BN). Far-field light is effectively coupled to the ultra-confined plasmon modes, demonstrating a new regime of light-matter interactions. Here, the spatial confinement of light extends the theoretical and practical understanding of plasmonics by minimizing damping through structured confinement systems.

Using advanced simulation techniques, including Finite-Difference-Time-Domain (FDTD) and semi-analytical methods, the paper conducted compares the local and non-local optical responses of materials employed. The results consistently validate the experimental framework through refined electric field distribution and plasmon resonance in the constructed systems. Notably, the research addresses non-local effects in metals, revealing significant implications on screening capabilities, further extending theoretical frameworks governing plasmonic behavior in nano-engineered systems.

The paper effectively illustrates the feasibility of leveraging van der Waals heterostructures as a groundwork for the sub-nanometer confinement of plasmons without principally compromising their lifetimes due to Landau damping. The underlying physics predicts the unprecedented ability to tune plasmon confinement using geometric adjustments and material specificity, significantly lowering optical losses.

This approach could have substantial practical implications, such as enhancements in light-matter interaction processes, the augmentation of molecular sensing due to heightened optical fields, and the development of high-efficiency photodetectors. Furthermore, the research opens avenues for viewing 2D-material heterostructures beyond conventional photonics applications, establishing foundational regimes applicable in diverse scientific domains including spectroscopic studies, sensing, quantum optics, and advanced photonic circuits.

The work progresses the understanding of light confinement in van der Waals heterostructure configurations, addressing the limits and dynamics involved. This could lead to further research into plasmonic modifications and their applications, augmenting both theoretical models and experimental setups in nanoscale photonics and material science. The pursuit of ultra-strong coupling regimes and low-loss applications stands poised to redefine paradigms within the field, prompting further explorations into the complex interplay between structure, material properties, and optical phenomena in nanoscale domains.

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