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Realization of the Axion Insulator State in Quantum Anomalous Hall Sandwich Heterostructures (1710.00471v2)

Published 2 Oct 2017 in cond-mat.mes-hall and cond-mat.mtrl-sci

Abstract: The 'magnetoelectric effect' arises from the coupling between magnetic and electric properties in materials. The Z2 invariant of topological insulators (TIs) leads to a quantized version of this phenomenon, known as the topological magnetoelectric (TME) effect. This effect can be realized in a new topological phase called an 'axion insulator' whose surface states are all gapped but the interior still obeys time reversal symmetry. We demonstrate such a phase using electrical transport measurements in a quantum anomalous Hall (QAH) sandwich heterostructure, in which two compositionally different magnetic TI layers are separated by an undoped TI layer. Magnetic force microscopy images of the same sample reveal sequential magnetization reversals of the top and bottom layers at different coercive fields, a consequence of the weak interlayer exchange coupling due to the spacer. When the magnetization is antiparallel, both the Hall resistance and Hall conductance show zero plateaus, accompanied by a large longitudinal resistance and vanishing longitudinal conductance, indicating the realization of an axion insulator state. Our findings thus show evidences for a phase of matter distinct from the established QAH state and provide a promising platform for the realization of the TME effect.

Citations (214)

Summary

  • The paper experimentally establishes the axion insulator state using QAH sandwich heterostructures with Cr- and V-doped topological insulator layers.
  • It employs electrical transport measurements and magnetic force microscopy to observe zero Hall conductance and verify a topological magnetoelectric response.
  • The study resolves previous ambiguities in axion insulator detection and suggests promising applications in quantum computing and spintronics.

Realization of the Axion Insulator State in Quantum Anomalous Hall Sandwich Heterostructures

The paper "Realization of the Axion Insulator State in Quantum Anomalous Hall Sandwich Heterostructures" presents an empirical exploration of novel material states within the domain of topological insulators, specifically targeting the axion insulator phase. This research centers on demonstrating the existence of an axion insulator state using quantum anomalous Hall (QAH) sandwich heterostructures composed of magnetically doped topological insulator (TI) layers with an undoped TI spacer.

The authors leverage the unique properties associated with the topological magnetoelectric (TME) effect inherent in axion insulators. Unlike conventional topological insulators which feature conducting surface states protected by time reversal symmetry, axion insulators maintain gapped surface states while preserving a θ=π topological invariant in their bulk. This specific configuration aligns with theoretical conditions necessary for observing the TME effect, characterized by a quantized response of electric polarization to applied magnetic fields, and vice versa.

Through meticulous experimental setup, the researchers constructed sandwich heterostructures comprising variably doped magnetic TI layers—specifically, a Cr-doped layer and a V-doped layer—separated by an undoped layer. A key experimental result identifying the axion insulator state was the observation of zero Hall conductance and zero Hall resistance plateaus in the magnetization antiparallel configuration. High longitudinal resistance in this state further corroborates the insulating behavior of the axion insulator, contrasting markedly with the QAH state marked by quantized Hall conductance.

The work stands out by effectively utilizing electrical transport measurements supplemented with magnetic force microscopy (MFM) to validate the antiparallel configuration of magnetization. The MFM results revealed distinct sequential magnetization reversals in the top and bottom layers as a result of the weak exchange coupling modulated by the spacer, leading to conditions conducive to an axion insulator state.

Furthermore, this paper addresses previous ambiguities reported in the literature concerning the realization of axion insulator states. It distinguishes between genuine axion insulators, arising from controlled magnetization alignments, and artifacts from measurement geometries or intrinsic magnetic domain scatterings in uniformly doped samples. By devising a heterostructure with different magnetic doping agents and systematically controlling chemical potentials, the authors assert satisfaction of the theoretical prerequisites for realizing axion insulators.

The implications of these findings are considerable. The experimental realization of axion insulator states paves the way for investigating rich phenomena like the TME effect and its potential applications in advanced electronic and spintronic devices. Future developments in AI might explore further engineering of heterostructures to facilitate the practical deployment of these topological phases, with the ultimate aim of integrating them into quantum computing systems and devices reliant on robust topological protection mechanisms.

In summary, this paper contributes a robust experimental framework and empirical evidence for the axion insulator state, presenting extensive data supporting the presence of this exotic phase with potential applications in topological quantum devices. This work lays a foundational basis for advancing the paper and exploitation of TME effects and broadening the understanding of topological materials.

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