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Multiple intrinsically identical single photon emitters in the solid-state (1310.3804v2)

Published 14 Oct 2013 in quant-ph, cond-mat.mtrl-sci, and physics.optics

Abstract: Emitters of indistinguishable single photons are crucial for the growing field of quantum technologies. To realize scalability and increase the complexity of quantum optics technologies, multiple independent yet identical single photon emitters are also required. However typical solid-state single photon sources are inherently dissimilar, necessitating the use of electrical feedback or optical cavities to improve spectral overlap between distinct emitters. Here, we demonstrate bright silicon-vacancy (SiV-) centres in low-strain bulk diamond which intrinsically show spectral overlap of up to 91% and near transform-limited excitation linewidths. Our results have impact upon the application of single photon sources for quantum optics and cryptography, and the production of next generation fluorophores for bio-imaging.

Citations (277)

Summary

  • The paper demonstrates that silicon-vacancy centers in ultrapure diamond achieve up to 91% spectral overlap with near transform-limited linewidths for consistent single photon emission.
  • The authors employ precise microwave plasma CVD techniques to control silicon doping at the ppb level, resulting in minimal spectral diffusion observed over 7 hours.
  • The findings support scalable quantum technologies by simplifying integration with photonic structures for applications in quantum cryptography, computing, and networking.

Overview of Multiple Intrinsically Identical Single Photon Emitters in the Solid-State

The paper "Multiple Intrinsically Identical Single Photon Emitters in the Solid-State" by L. J. Rogers et al. explores the development of indistinguishable single-photon sources, which are pivotal for various quantum technologies. The authors address a significant challenge in solid-state quantum emitters: achieving intrinsic uniformity in spectral properties without external tuning mechanisms such as optical cavities or electrical feedback.

Key Contributions

  • Silicon-Vacancy (SiV^-) Centers: The authors demonstrate that SiV^- centers embedded in low-strain, ultrapure diamond substrates can yield single-photon emissions with remarkably high spectral overlap, up to 91%. These emissions possess near transform-limited linewidths, signifying minimal spectral diffusion and high fidelity photon production over extended periods.
  • Experimental Results: The paper explores the homogeneous nature of the SiV^- centers by evaluating both the linewidth and the spectral position of the emissions. The linewidths show minimal deviation beyond the transform-limit, with negligible spectral diffusion observed over a 7-hour period. This uniformity is further evidenced by photoluminescent excitation (PLE) spectra from various closely spaced SiV^- centers, revealing differences in line position well within one transform-limited linewidth for more than half of the pairs studied.
  • Meticulous Sample Preparation and Characterization: The methodology entails high precision in diamond sample preparation through microwave plasma chemical vapor deposition (MPCVD). Silicon doping is controlled to the ppb level to ensure consistent incorporation of SiV^- centers. Confocal microscopy and spectroscopy are used to ascertain the emission characteristics, highlighting their stability and uniformity.

Implications and Future Directions

The evidence gathered showcases SiV^- centers as feasible candidates for scalable quantum technologies. These intrinsically identical photon sources can be pivotal in applications such as quantum cryptography, linear optical quantum computing, and quantum repeaters. The inherent stability and narrow linewidths of these emitters potentially reduce the complexity associated with external stabilization mechanisms, thus simplifying integration processes in quantum devices.

Looking forward, the broader adoption of SiV^- centers could influence the design of quantum networks, favoring architectures where multiple identical photon sources are critical. Additionally, the successful coupling of these emitters with photonics structures like nano-cavities or waveguides might further enhance their applicability in quantum optics.

Challenges and Considerations

While the results are promising, the potential impact of residual impurities and their influence on emitter homogeneity over larger scales warrants attention. Furthermore, the paper leaves room for exploring how SiV^- centers might interact with other quantum systems, such as spin-based qubits for information processing. A better understanding of these interactions could open pathways to more complex quantum states and operations that are vital for advanced quantum computing applications.

Conclusion

L. J. Rogers et al. have presented an insightful exploration of SiV^- centers as uniform single-photon sources within a solid-state environment. Their findings reinforce the notion that achieving intrinsic identicalness in photon emissions is not only feasible but can pave the way for practical and scalable quantum technologies. Continued research could unlock further potential in this domain, positioning SiV^- centers as a foundational element in future quantum optics infrastructures.

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