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Inertial effects in ultrafast spin dynamics (2303.15251v2)

Published 27 Mar 2023 in cond-mat.other and cond-mat.mes-hall

Abstract: The dynamics of magnetic moments consist of a precession around the magnetic field direction and a relaxation towards the field to minimize the energy. While the magnetic moment and the angular momentum are conventionally assumed to be parallel to each other, at ultrafast time scales their directions become separated due to inertial effects. The inertial dynamics give rise to additional high-frequency modes in the excitation spectrum of magnetic materials. Here, we review the recent theoretical and experimental advances in this emerging topic and discuss the open challenges and opportunities in the detection and the potential applications of inertial spin dynamics.

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Summary

  • The paper demonstrates that incorporating an inertial term into the LLG model reveals high-frequency nutational modes beyond conventional precession.
  • It employs numerical simulations and theoretical analysis to show a redshifted precessional resonance in ferromagnetic dynamics.
  • Experimental pump-probe techniques in materials like NiFe and CoFeB support these findings, highlighting potential applications in ultrafast spintronics.

Inertial Effects in Ultrafast Spin Dynamics

The paper "Inertial effects in ultrafast spin dynamics" provides a comprehensive examination of the influence of inertial dynamics on the behavior of magnetic moments at ultrafast time scales. The authors explore how these inertial effects introduce novel, high-frequency modes in magnetic materials, challenging the conventional assumption that magnetic moments and angular momentum are parallel and can instantaneously adjust to each other. This paper thoroughly reviews theoretical developments and experimental efforts in this burgeoning field, highlighting both challenges in detecting inertial dynamics and potential applications that could arise from these insights.

Theoretical and Experimental Insights

The dynamics of magnetic moments are typically described by the Landau-Lifshitz-Gilbert (LLG) equation, which accounts for the precession around an external magnetic field and relaxation or damping towards minimizing energy. However, on ultrafast time scales, this traditional model is insufficient to describe the inertia between the magnetic moment and its angular momentum, particularly when viewed in the context of femto- and picosecond dynamics.

To accommodate these high-speed dynamics, the LLG equation is augmented with an inertial term that features a second time derivative of the magnetization. This addition fundamentally changes the dynamics, introducing nutation—a high-frequency oscillation separate from the more commonly considered precession of the magnetic moment. The inertial effects give rise to nutational resonance peaks within the terahertz range, in contrast to conventional GHz-range precession peaks.

Numerical and Analytical Findings

The authors explore the implications of this revised inertial LLG (ILLG) model on both ferromagnetic resonance (FMR) and spin-wave dynamics using numerical simulations and theoretical analyses. They conclude that the inertia introduces a notable redshift in the precessional resonance frequency and predicts a distinct nutational resonance in the high-frequency spectrum. This nutational resonance is an essential confirmation of the inertial model, as traditional LLG dynamics cannot account for such high-frequency responses.

Experimental Observations

A significant part of the paper highlights recent experimental observations that align with theoretical predictions. Notably, experiments using time-resolved magneto-optical pump-probe techniques have identified high-frequency responses in various magnetic materials like NiFe and CoFeB, corroborating the presence of nutational dynamics. However, the community recognizes a need for further experimental work to unequivocally establish the inertial effects across different materials and conditions.

Implications and Future Directions

The recognition of inertial dynamics could pave the way for ultrafast magnetic technology, where magnetic moments are manipulated with unprecedented speed and precision. This has potential applications in data storage and processing technologies, where speed and efficiency are critical. However, the field is confronted with theoretical and experimental challenges, primarily regarding the precise characterization of inertial parameters and understanding their behavior in complex magnetic systems.

Emphasizing future research avenues, the paper suggests that optical methods given their natural frequency range, might prove exceptionally beneficial for probing nutational dynamics. Moreover, antiferromagnets, with their characteristic high-frequency precessional modes, present a particularly promising platform for experimental exploration of inertial dynamics, especially given that nutational and precessional modes in these materials can coexist within the same frequency regime, thus amenable to concurrent analysis.

Conclusion

The exploration of inertial effects in magnetic dynamics represents an exciting frontier with theoretical intrigue and technological promise. As experimental realism aligns with theoretical predictions, the potential for these effects to redefine the parameters of ultrafast magnetism becomes increasingly tenable. The paper serves as a call to action for continued research, fostering a deeper understanding of spin dynamics on the fastest time scales accessible, and advancing the manipulation of spintronics beyond today's technological frontiers.

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