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Direct observation of the Dzyaloshinskii-Moriya interaction in a Pt/Co/Ni film (1409.8570v2)

Published 30 Sep 2014 in cond-mat.mtrl-sci and cond-mat.mes-hall

Abstract: The interfacial Dzyaloshinskii-Moriya interaction (DMI) in an in-plane anisotropic Pt(4nm)/Co(1.6nm)/Ni(1.6nm) film has been directly observed by Brillouin spectroscopy. It is manifested in the asymmetry of the measured magnon dispersion relation, from which the DMI constant has been evaluated. Linewidth measurements reveal that the lifetime of the magnons is asymmetric with respect to their counter-propagating directions. The lifetime asymmetry is dependent on the magnon frequency, being more pronounced the higher the frequency. Analytical calculations of the magnon dispersion relation and linewidth agree well with experiments.

Citations (248)

Summary

  • The paper directly observes the Dzyaloshinskii–Moriya interaction in a Pt/Co/Ni film using Brillouin light scattering to reveal pronounced asymmetries in magnon dispersion.
  • Experimental results quantify the DMI constant at approximately 0.44 mJ/m² and highlight direction-dependent magnon lifetimes that align with analytical models.
  • These findings advance the development of nonreciprocal magnonic devices and efficient spintronic applications by leveraging chiral magnetic structures.

Direct Observation of the Dzyaloshinskii-Moriya Interaction in a Pt/Co/Ni Film

The investigation detailed in the paper "Direct observation of the Dzyaloshinskii-Moriya interaction in a Pt/Co/Ni film" provides valuable empirical insight into the interfacial Dzyaloshinskii-Moriya Interaction (DMI) by employing Brillouin light scattering (BLS) techniques. This paper confirms the presence of DMI in a Pt(4nm)/Co(1.6nm)/Ni(1.6nm) film, a topic of substantial significance given its fundamental role in chiral magnetic structures and potential applications in spintronics technologies.

One of the paper's primary accomplishments is the direct observation of a pronounced asymmetry in the magnon dispersion relation in this multilayer structure, which serves as evidence of DMI at the Pt/Co interface. The DMI constant calculated was approximately 0.44 mJ/m², providing a quantitative measure of the interaction's strength. This work demonstrates that BLS is a suitable method for detecting DMI in multilayers, where traditional techniques like spin-polarized electron energy loss spectroscopy and inelastic neutron scattering are less effective.

Experimental results revealed that magnon lifetimes are direction-dependent, exhibiting asymmetry in lifetime that increases with frequency. The analysis showed the calculated magnon dispersion relation and linewidth are coherent with experimental data, reinforced by the use of analytical calculations. The linewidth variation observed suggests the presence of an antisymmetric term in the dispersion relation due to DMI.

Understanding the interfacial DMI has significant implications for developing nonreciprocal magnonic devices such as spin-wave isolators in microwave technology. These asymmetric magnonic features can be controlled or manipulated, offering a pathway to advance high-density memory applications and efficient spintronic devices. Additionally, the insights into magnon lifetime asymmetries induced by DMI can be vital for optimizing spin-wave coherence in magnonic circuits.

Moreover, the findings correlate with broader efforts to miniaturize and enhance the efficiency of magnonic circuits, leveraging the chirality introduced by DMI. The pronounced linear relationship between the frequency differences of counter-propagating spin-waves with the wave vector offers prospects for integrated magnonic circuits that capitalize on wave interference and dispersion characteristics.

In conclusion, this paper provides robust experimental evidence for the existence of interfacial DMI in Pt/Co/Ni multilayers. This advances the understanding of spin-wave dynamics in these structures and opens avenues for the development of advanced spintronics and magnonic devices. Future work could explore the tuning of DMI through interface engineering and its implications on control over chiral magnetic textures. Such advancements could further exploit DMI for emerging memory technologies and ultra-low energy electronic applications.

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