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Spin-Hall conductivity and optical characteristics of noncentrosymmetric quantum spin Hall insulators: the case of PbBiI (2405.03655v2)

Published 6 May 2024 in cond-mat.mes-hall

Abstract: Quantum spin Hall insulators have attracted significant attention in recent years. Understanding the optical properties and spin Hall effect in these materials is crucial for technological advancements. In this study, we present theoretical analyses to explore the optical properties, Berry curvature and spin Hall conductivity of pristine and perturbed PbBiI using the linear combination of atomic orbitals and the Kubo formula. The system is not centrosymmetric and it is hosting at the same time Rashba spin-splitting and quantized spin Hall conductivity. Our calculations reveal that the electronic structure can be modified using staggered exchange fields and electric fields, leading to changes in the optical properties. Additionally, the spin Berry curvature and spin Hall conductivity are investigated as a function of the energy and temperature. The results indicate that due to the small dynamical spin Hall conductivity, generating an ac spin current in PbBiI requires the use of external magnetic fields or magnetic materials.

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