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Decoupling superconductivity and correlated insulators in twisted bilayer graphene (1911.13302v2)

Published 29 Nov 2019 in cond-mat.mes-hall, cond-mat.mtrl-sci, cond-mat.str-el, and cond-mat.supr-con

Abstract: When bilayer graphene is rotationally faulted to an angle $\theta\approx 1.1\circ$, theory predicts the formation of a flat electronic band and correlated insulating, superconducting, and ferromagnetic states have all been observed at partial band filling. The proximity of superconductivity to correlated insulators has suggested a close relationship between these states, reminiscent of the cuprates where superconductivity arises by doping a Mott insulator. Here, we show that superconductivity can appear without correlated insulating states. While both superconductivity and correlated insulating behavior are strongest near the flat band condition, superconductivity survives to larger detuning of the angle. Our observations are consistent with a "competing phases" picture, in which insulators and superconductivity arise from disparate mechanisms.

Citations (375)

Summary

  • The paper demonstrates that superconductivity in tBLG is independent of correlated insulating states, challenging traditional views of their interdependence.
  • It utilizes controlled experiments with the cut-and-stack method to reduce strain, revealing a robust superconducting phase even when insulator signals weaken.
  • Findings indicate that superconductivity arises from a high density of states at the Fermi level, distinct from the mechanisms governing correlated insulators.

Decoupling Superconductivity and Correlated Insulators in Twisted Bilayer Graphene

The research presented focuses on the distinct manifestations of superconductivity and correlated insulating behaviors within twisted bilayer graphene (tBLG) at a specific twist angle close to the "magic angle" of 1.1°. The paper challenges the hypothesis that the proximity of superconductivity in tBLG to correlated insulator states necessarily indicates a derivation of one state from the other. By exploring the structural and electronic properties of tBLG through meticulous experiments involving multiple devices, the paper presents strong evidence that superconductivity in tBLG can manifest independently of the presence of correlated insulating behavior.

The investigators employ a variety of experimental techniques to scrutinize devices fabricated under varying conditions, identifying a superconducting phase that persists even when typical correlated insulating behavior is absent at integer band filling. Superconductivity in this context is starkly apparent due to a transition to low resistivity states at low temperatures and features associated with superconducting junctions, such as Fraunhofer-like patterns.

By examining superconducting devices fabricated with the "cut-and-stack" method to minimize strain and inhomogeneity, the paper illustrates the robustness of superconductivity across a range of twist angles, with a peak in critical temperature observed near the magic angle. Noteworthy is that superconductivity is achieved even as the insulator phase weakens or disappears entirely, drawing a clear line of distinction between these phases. The results support a "competing phases" paradigm rather than a cooperative one, indicating the phases arise from distinctly separate mechanisms.

Furthermore, the work speculates on the theoretical implications of these observations. It posits that, unlike the correlated insulating states that necessitate extreme band narrowness to align with a Stoner criterion for spontaneous symmetry breaking, the superconductivity leverages the high density of states at the Fermi level intrinsic to near-magic angle tBLG. Hence, superconductivity may be more resilient to deviations from the ideal angle because its underlying mechanism might align more closely with conventional electron-phonon interactions.

The practical consequences of this paper are profound, offering expanded use cases for tBLG in applications that might decouple the advantages of superconductivity from correlated insulator behaviors. Theoretically, it suggests a potential reevaluation of the roles different interactions play in complex electron systems. The decoupling of superconductivity and correlated insulators sets a foundation for future explorations into novel electronic phases accessible through precise tuning of the moiré superlattice parameters.

In conclusion, this research not only clarifies the nature of superconductivity in twisted bilayer graphene but also provides an essential roadmap for approaching the synthesis and manipulation of electron phases in complex quantum materials.

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