Tension-Induced Soft Stress and Viscoelastic Bending in Liquid Crystal Elastomers for Enhanced Energy Dissipation (2506.23360v1)

Abstract: Architected materials that harness elastic snap-through buckling can trap energy reversibly. Liquid crystal elastomers (LCEs) exhibit excellent dissipation capabilities due to polymer network viscoelasticity and rate-dependent soft stress behavior associated with mesogen rotation. Incorporating LCEs into buckling lattice structures enhances energy absorption; however, conventional design cannot take advantage of the dissipation mechanism associated with mesogen rotation because buckling occurs at strains below the threshold of the soft stress response. In this study, we investigate tension-induced mesogen rotation as an additional dissipation mechanism in horizontal members of structures composed of tilted LCE beams under compression. Viscoelastic properties of LCEs with two crosslinking densities were characterized experimentally, and a nonlinear viscoelastic user-defined element was implemented in Abaqus/Standard to capture finite-strain behavior, including soft stress effects. Simulations and experiments revealed a non-monotonic dependence of energy dissipation on the thickness ratio between horizontal and tilted LCE members. Optimized structures with stretchable horizontal bars dissipated 2-3 times more energy than rigid-bar counterparts by balancing tension-driven soft stress with viscoelastic beam bending. Energy contributions from mesogen rotation and polymer network viscoelasticity were quantified. These findings inform the design strategies for LCE-based architected materials to enhance dissipation.