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Momentum-dependent electron-phonon coupling in cuprates by RIXS: the roles of phonon symmetry and electronic structure (2501.12089v3)

Published 21 Jan 2025 in cond-mat.str-el

Abstract: The experimental determination of the magnitude and momentum dependence of electron-phonon coupling (EPC) is an outstanding problem in condensed matter physics. Resonant inelastic x-ray scattering (RIXS) has been previously employed to determine the EPC, since the intensity of phonon peaks in RIXS spectra has been directly related to the underlying EPC strength. In order to assess the limits of validity of such a relation, we compare experimental results and theoretical predictions for several high-T$c$ superconducting cuprates. Namely, we investigate the intensity of the bond-stretching phonon mode in CaCuO$_2$, La$_2$CuO${4+\delta}$, La${1.84}$Sr${0.16}$CuO$4$ and YBa$_2$Cu$_3$O${7-\delta}$ along the high symmetry ($\zeta$,0), ($\zeta$,$\zeta$) directions and as a function of the azimuthal angle $\phi$ at fixed modulus of the in-plane momentum $\mathbf{q_\parallel}$. Using two different theoretical approaches for the description of the RIXS scattering from phonons, we find that the $\mathbf{q_\parallel}$-dependence of the RIXS intensity can be largely ascribed to the symmetry of the phonon mode, and that satisfactory prediction of the experimental results cannot be obtained without including realistic details of the electronic structure in the calculations. Regardless of the theoretical model, RIXS provides a reliable momentum dependence of EPC in cuprates and can be used to test advanced theoretical predictions.

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