Scale-invariant magnetic anisotropy in $α$-RuCl$_3$: A quantum Monte Carlo study (2312.03080v1)

Abstract: We compute the rotational anisotropy of the free energy of $\alpha$-RuCl$_3$ in an external magnetic field. This quantity, known as the magnetotropic susceptibility, $k$, relates to the second derivative of the free energy with respect to the angle of rotation. We have used approximation-free, auxiliary-field quantum Monte Carlo simulations for a realistic model of $\alpha$-RuCl$_3$ and optimized the path integral to alleviate the negative sign problem. This allows us to reach temperatures down to $30~\rm{K}$ -- an energy scale below the dominant Kitaev coupling. We demonstrate that the magnetotropic susceptibility in this model of $\alpha$-RuCl$_3$ displays unique scaling, $k = Tf(B/T)$, with distinct scaling functions $f$ at high and low temperatures. In comparison, for the XXZ Heisenberg model, the scaling $k = Tf(B/T)$ breaks down at a temperature scale where the uniform spin susceptibility deviates from the Curie law (i.e. at the energy scale of the exchange interactions) and never recovers at low temperatures. Our findings suggest that correlations in $\alpha$-RuCl$_3$ lead to degrees of freedom that respond isotropically to a magnetic field. One possible interpretation for the apparent scale-invariance observed in experiments could be fractionalization of the spin degrees of freedom in the extended Kitaev model.