Dynamically tunable moiré Rydberg excitons in a monolayer semiconductor on twisted bilayer graphene (2303.08980v1)

Abstract: Moir\'e excitons are emergent optical excitations in 2D semiconductors with deep moir\'e superlattice potentials. While these excitations have been realized in several platforms, a system with dynamically tunable moir\'e potential to tailor the moir\'e exciton properties is yet to be realized. Here, we present a continuously tunable moir\'e potential in a monolayer WSe2 that is enabled by its proximity to twisted bilayer graphene (TBG) near the magic-angle. Due to its flat electronic bands, charge distribution is highly localized and forms a triangular lattice in TBG. Tuning the local charge density via electrostatic gating, TBG thus provides a spatially varying and dynamically tunable dielectric superlattice for modulating monolayer exciton wavefunctions. By performing optical reflection spectroscopy, we observe emergent moir\'e exciton Rydberg branches in monolayer WSe2 with increased energy splitting upon doping TBG. The twist-angle dependence reveals that the observation is due to a hybridization between bright and dark Rydberg states enabled by the moir\'e potential. Further, at the magic-angle near 1.1{\deg}, the moir\'e Rydberg excitons form a sawtooth pattern with doping owing to the formation of strongly correlated states in the TBG. Our study provides a new platform for engineering moir\'e excitons as well as optical accessibility to the electronic states with small correlation gaps in TBG.