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Giant Rydberg Excitons in Cuprous Oxide (1407.0691v1)

Published 2 Jul 2014 in cond-mat.mes-hall, cond-mat.mtrl-sci, and physics.atom-ph

Abstract: Highly excited atoms with an electron moved into a level with large principal quantum number are fascinating hydrogen-like objects. The giant extension of these Rydberg atoms leads to huge interaction effects. Monitoring these interactions has provided novel insights into molecular and condensed matter physics problems on a single quantum level. Excitons, the fundamental optical excitations in semiconductors consisting of a negatively charged electron and a positively charged hole, are the condensed matter analogues of hydrogen. Highly excited excitons with extensions similar to Rydberg atoms are attractive because they may be placed and moved in a crystal with high precision using microscopic potential landscapes. Their interaction may allow formation of ordered exciton phases or sensing of elementary excitations in the surrounding, also on a quantum level. Here we demonstrate the existence of Rydberg excitons in cuprous oxide, Cu2O, with principal quantum numbers as large as n=25 . These states have giant wave function extensions of more than 2 micrometers, compared to about a nanometer for the ground state. The strong dipole-dipole interaction is evidenced by a blockade effect, where the presence of an exciton prevents excitation of a further exciton in its vicinity.

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