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Bright single-photon sources in bottom-up tailored nanowires (1203.5676v1)

Published 26 Mar 2012 in cond-mat.mes-hall and physics.optics

Abstract: The ability to achieve near-unity light extraction efficiency is necessary for a truly deterministic single photon source. The most promising method to reach such high efficiencies is based on embedding single photon emitters in tapered photonic waveguides defined by top-down etching techniques. However, light extraction efficiencies in current top-down approaches are limited by fabrication imperfections and etching induced defects. The efficiency is further tempered by randomly positioned off-axis quantum emitters. Here, we present perfectly positioned single quantum dots on the axis of a tailored nanowire waveguide using bottom-up growth. In comparison to quantum dots in nanowires without waveguide, we demonstrate a 24-fold enhancement in the single photon flux, corresponding to a light extraction efficiency of 42 %. Such high efficiencies in one-dimensional nanowires are promising to transfer quantum information over large distances between remote stationary qubits using flying qubits within the same nanowire p-n junction.

Citations (421)

Summary

  • The paper demonstrates a novel bottom-up nanowire fabrication method that achieves 42% photon extraction efficiency with precise on-axis quantum dot placement.
  • The methodology employs tapered waveguide design and a post-growth gold mirror to boost single-photon flux by 24-fold.
  • The findings underpin advances in scalable quantum photonic technologies, offering pathways toward efficient quantum communication systems.

Bright Single-Photon Sources in Bottom-Up Tailored Nanowires

The paper presents a significant advancement in achieving high-efficiency single-photon emission through an innovative bottom-up fabrication approach of nanowire waveguides containing single quantum dot (QD) emitters. This work addresses the limitations inherent in traditional top-down etching methods, such as fabrication imperfections, etching-induced defects, and the misalignment of quantum dots (QDs) relative to the optical axis of waveguides, which affect the quantum efficiency and light extraction efficiency of single-photon sources.

Overview and Results

The authors report on the growth of InAsP QDs positioned axially within InP nanowire waveguides using a bottom-up growth technique. This method allows precise control over both the nanowire shape and QD location. The nanowires are tailored to exhibit a tapering geometry towards the tip, optimizing the light extraction while maintaining the quantum dot exactly on-axis. The tailored geometry incorporates a waveguide section where the QD is optimally positioned, with a minimal taper angle facilitating efficient single-photon emission into the waveguide's fundamental mode. Additionally, they implement a bottom gold mirror technique post-growth to reflect downward-emitted photons, thereby enhancing photon collection.

The authors demonstrate a 24-fold enhancement in single-photon flux compared to previous standard nanowires, reaching a photon extraction efficiency of 42% at the first optical lens. This represents a substantial step forward in the proper coupling of quantum emission into controlled optical modes, crucial for developing scalable quantum technologies.

Experimental and Theoretical Implications

From an experimental standpoint, this paper underscores the advancement in nanofabrication techniques, particularly the AI-driven control of nanoscale material properties through bottom-up growth methods. The achievement of near-perfect on-axis placement of quantum dots illustrates the precise control required over growth conditions, making it feasible to fabricate highly efficient quantum light sources.

On the theoretical side, the results have implications for quantum electrodynamics (QED) within photonic structures, as this work demonstrates how tailored waveguide designs can enhance the light-matter interaction by controlling mode structures and emitter positioning precisely. The utilization of finite-difference time-domain (FDTD) simulations offers insights into optimizing light extraction efficiencies by manipulating waveguide geometries and refractive index contrasts.

Future Prospects

Looking forward, the research sets a precedent for further advancements in quantum information transfer technologies. The integration into nanowire p-n junctions for remote qubit communication suggests potential applications in quantum computing networks and quantum internet development. Future work could explore integrating these nanowires into hybrid photonic circuits and optimizing reflective coatings to further enhance modal reflectivity and overall efficiency.

Additionally, solving the challenges related to emitter-electrode coupling and charge state control could lead to robust single-photon sources for use in scalable quantum cryptographic systems and high-resolution quantum sensing. Continued exploration of different materials and alloy compositions using similar bottom-up techniques might yield even higher efficiencies and broader wavelength applicability, opening new frontiers in photonics and quantum information science.

In conclusion, the paper exhibits a meticulous alignment of experimental methodologies with theoretical models, pushing the boundaries of quantum light source technologies. The bottom-up approach for fabricating tailored nanowire waveguides with precisely positioned quantum emitters marks a meaningful stride forward toward practical quantum photonics applications.