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A KInetic Database for Astrochemistry (KIDA) (1201.5887v1)

Published 27 Jan 2012 in astro-ph.GA

Abstract: We present a novel chemical database for gas-phase astrochemistry. Named the KInetic Database for Astrochemistry (KIDA), this database consists of gas-phase reactions with rate coefficients and uncertainties that will be vetted to the greatest extent possible. Submissions of measured and calculated rate coefficients are welcome, and will be studied by experts before inclusion into the database. Besides providing kinetic information for the interstellar medium, KIDA is planned to contain such data for planetary atmospheres and for circumstellar envelopes. Each year, a subset of the reactions in the database (kida.uva) will be provided as a network for the simulation of the chemistry of dense interstellar clouds with temperatures between 10 K and 300 K. We also provide a code, named Nahoon, to study the time-dependent gas-phase chemistry of 0D and 1D interstellar sources.

Citations (408)

Summary

  • The paper introduces a curated astrochemical database that unifies experimental and theoretical gas-phase reaction rates and their uncertainties.
  • It details comprehensive chemical species data and reaction parameters, enabling accurate modeling across varied astronomical environments.
  • The resource supports efficient computational analysis through integrated tools like the Nahoon code and promises broader interoperability with future platforms.

A Kinetic Database for Astrochemistry (KIDA)

The paper entitled "A KInetic Database for Astrochemistry (KIDA)" introduces a comprehensive and meticulously curated chemical database catering to the needs of astrochemical modeling. This resource is critical for researchers modeling the chemical processes occurring in various astronomical environments, namely the interstellar medium (ISM), planetary atmospheres, and circumstellar envelopes. The KIDA database is a repository of gas-phase reactions, offering vetted rate coefficients and associated uncertainties, which are essential for the development and refinement of chemical models.

Key Features of KIDA

KIDA distinctly provides a platform for merging experimental and theoretical results regarding rate coefficients and their uncertainties. Its structure allows users to submit their measured or computed data, which are thoroughly analyzed by domain experts before inclusion. The database is designed for effective data management, augmented by user-friendly visualization and the flexible downloading of reaction lists pertinent to specific research needs.

The structure of KIDA embraces:

  • Chemical Species Data: This includes details such as InChI codes, CAS registry numbers, electronic states, polarizability index, dipole moments, and enthalpy of formation.
  • Rate Coefficients: These are pivotal to defining the kinetics of gas-phase reactions, recorded with specific parameters (A, B, C) to accommodate different temperature dependencies across nine reaction categories.

Implications and Future Prospects

The creation of KIDA seeks to synchronize the efforts in astrochemical research, providing a standardized and critical resource that minimizes the disparities seen in pre-existing databases like the UMIST Database for Astrochemistry (udfa) and the database previously developed by Eric Herbst and collaborators at Ohio State University (OSU). This initiative implies a significant shift towards uniformity and reliability in astrochemical data, enhancing the accuracy of chemical models used in studies of ISM and planetary atmospheres.

With its implication divergent from existing resources, KIDA aims to unify astrochemical data, thus fostering better model predictions and facilitating novel discoveries within this domain. Moreover, this endeavor anticipates a scaling expansion, which will integrate reaction networks tailored towards understanding circumstellar chemistry and planetary atmospheres.

Additionally, KIDA is set to expand its repertoire by eventually including data on state-to-state dynamics, isotopologues, and potentially distinguished ortho and para forms of molecules. An anticipated integration with platforms such as the Virtual Atomic and Molecular DataCenter (VAMDC) is expected to improve the reach and interoperability of KIDA among various scientific repositories and communities.

Modeling and Computational Tools

Accompanying KIDA's database is the Nahoon numerical code, intended for computational analysis of gas-phase chemistry in 0D and 1D astrophysical contexts. This software aligns with the data structures from KIDA, enabling simulations that account for temperature-dependent reaction networks. An added feature is the ability to calculate reaction rates without extrapolating beyond validated temperature ranges, ensuring the integrity of simulations and observational comparisons.

Conclusion

KIDA exemplifies an ambitious effort to centralize and critique the chemical kinetic data vital for understanding astrochemical processes. It reflects ongoing advancements in the field, offering a strategic approach to integrating experimental and theoretical results across multiple domains of interest within astrochemistry. As the initiative progresses, KIDA will undoubtedly play a transformative role, paving the way for deeper insights into complex chemical phenomena in varied astronomical contexts.